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Dr. Yuan Gao
Associate Professor, Atmospheric Chemistry
Phone: (973) 353-1139
Fax: (973) 353-1965
Email: yuangaoh@andromeda.rutgers.edu
Mailing Address:
Department of Earth and Environmental Sciences
Rutgers University
101 Warren Street
Newark, NJ 07102
USA
Additional Affiliation:
Institute of Marine and Coastal Sciences
Rutgers University New Brunswick
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Education>>
- PhD, Oceanography, University of Rhode Island, 1994
Graduate Advisor: Professor Robert A. Duce
Research Areas>>
Characterization of Atmospheric Dust Properties through Field/Laboratory Experiments
As an aerosol, dust affects the Earth's radiation budget through direct and indirect effects. The degrees of both effects are dominated by chemical and physical properties of dust. Dust particles also provide reaction sites for many heterogeneous reactions involving SO2, NOy, HOx, O3, etc. and serve as conveyors carrying anthropogenic substances from the continents to the remote environments through the long-range transport. Those processes may alter the chemical and physical properties of dust (including aeolian iron solubility and then its bioavailability to the surface ocean biota). Characterization of dust properties is thus crucially important to quantify dust climate forcing and to understand its biological role in the ocean biogeochemical cycles. Our work in this direction includes field and laboratory efforts, reflected by selected publications below:
- Gao, Y., R. Arimoto, R. A. Duce, D. S. Lee, and M. Y. Zhou, Input of atmospheric trace elements and mineral matter to the Yellow Sea during the spring of a low dust year, Journal of Geophysical Research, 97, 3767 - 3777, 1992.
- Gao, Y., R. Arimoto, M. T. Zhou, J. T. Merrill, and R. A. Duce, Relationships between the dust concentrations over eastern Asia and the remote North Pacific, Journal of Geophysical Research, 97, 9867 - 9872, 1992.
- Gao, Y., R. Arimoto, R. A. Duce, M. Y. Zhou, L. Q. Chen, X. Y. Zhang, G. Y. Zhang, and Z. S. An, Temporal and spatial distribution of dust and its total deposition to the China Sea, Tellus, 49B, 172 - 189, 1997.
- Gao, Y., and J. Anderson, Characteristics of Chinese aerosols determined by individual-particle analyses, Journal of Geophysical Research, 106, 18,037-18045, 2001.
- Gao, Y., J.R. Anderson, and X. Hua, Dust characteristics over the North Pacific observed through shipboard measurements during the ACE-Asia Experiment, Atmospheric Environment, 41,7907-7922, 2007.
- Xu, N, and Y. Gao, Characterization of hematite dissolution affected by oxalate coating, kinetics and pH, Applied Geochemistry, 23, 783-793, 2008.
Quantifying Atmospheric Iron Input to the Ocean through Modeling and Data Assimilations
Dust is a source of iron, an essential micronutrient for phytoplankton growth in the surface ocean. Recent Fe fertilization experiments conducted in the HNLC ocean waters confirmed that Fe supplies strongly regulate phytoplankton growth in certain oceanic regions. The atmospheric Fe input may, in turn, regulate the global carbon cycle and thus affect climate. In particular, at present, climate warming has caused increased stratification in the upper ocean that may prevent the surface ocean from mixing with the deep ocean and decrease the nutrient fluxes from below, oceanic primary production could be more dependent on the nutrient input from external sources, such as atmospheric Fe deposition. Therefore, quantifying atmospheric iron deposition to the ocean is important. Our work in this direction has been made through modeling and data assimilations integrated with remote sensing; examples of our efforts are:
- Gao, Y., Y. J. Kaufman, D. Tanre, D. Kolber, and P. G. Falkowski, Seasonal distributions of aeolian iron fluxes to the global ocean, Geophysical Research Letters, 28, 29-32, 2001.
- Gao, Y., S-M Fan, and J. L. Sarmiento, Aeolian iron input to the ocean through precipitation scavenging: A modeling perspective and its implication for natural iron fertilization in the ocean, Journal of Geophysical Research, 108, 2003.
- Yang, H., and Y. Gao, Air-to-sea flux of soluble iron: Is it driven more by HNO3 or SO2? - An examination in the light of dust aging, Atmospheric Chemistry and Physics Discussions, 7, 10043-10063, 2007.
Characterization of Atmospheric Nitrogen Deposition to Coastal Waters through Field Measurements
The coastal marine atmosphere adjacent to or downwind of large urban and industrial centers can be strongly impacted by pollution emissions, and high concentrations of pollutants in coastal air could result in enhanced air-to-sea deposition fluxes. One of the consequences is accelerated coastal primary production (or eutrophication) driven by excessive discharges of nutrient nitrogen (N) from both point and non-point sources, such as atmospheric deposition. With earlier work on the Asian coast, we recently have focused on quantifying atmospheric nitrogen over the US East Coast, in particular atmospheric nitrogen deposition to the New Jersey coastal ecosystems on the coast of the Mid-Atlantic Bight. Detailed results are in:
- Gao, Y, R. Arimoto, R. A. Duce, L. Q. Chen, M. Y. Zhou, and D. Y. Gu, Atmospheric non-sea-salt sulfate, nitrate, and methanesulfonate over the China Sea, Journal of Geophysical Research, 101, 12,601-12,611, 1996.
- Gao, Y., Atmospheric nitrogen deposition to Barnegat Bay, Atmospheric Environment, 36, 5783-5794, 2002.
- Ayars, J., and Y. Gao, Atmospheric nitrogen deposition to the Mullica River-Great Bay Ecosystem, Marine Environmental Research, 64, 590-600, 2007.
- Gao, Y., M. Kennish, and A.M. Flynn, Atmospheric deposition of nitrogen to New Jersey coastal waters and its implications for nutrient enrichment and biotic impacts, Journal of the Ecological Society of America, S31-S41, 2007.
Urban Air Pollution Characterization through Ambient Measurements
Urban air pollution has drawn increasing attention due to its impacts on air quality, human health, and regional and global climate change. Air pollutants, both primary and secondary, may exist in aerosol-, gas-, and precipitation- phases, functioning differently. Therefore air quality represents a result of interactions of different air components and environmental factors. Our efforts in the area of urban air pollution characterization are mainly based at Newark, the largest metropolitan center in New Jersey and adjacent to New York City. Examples of our efforts are as follows:
- Zhao, Y, and Y. Gao, Mass size distributions of water-soluble inorganic and organic ions in size segregated aerosols over metropolitan Newark in the US East Coast, Atmospheric Environment, 42, 4063 - 4078, 2008.
- Zhao, Y, and Y. Gao, Acidic species and chloride depletion in coarse aerosol particles in the US east coast, Science of the Total Environment, 407, 541-547, 2008.
- Song, F., and Y. Gao, Chemical characteristics of precipitation at metropolitan Newark in the US East Coast, Atmospheric Environment, in press, 2009.
Research Group Members>>
- Fei Song, PhD student (MS, Marine Chemistry, Chinese Academy of Sciences)
- Rafael Jusino-Atresino, PhD student (MS, Natural Sciences, Texas Tech University)
- Lili Xia, PhD student (MS, Quaternary Geology, Peking University, China)
- Lu Wang, PhD student (MS, Oceanography, Dalhousie University, Canada)
- Christopher Thuman, MS student (BS, Meteorology, State University of New York)
- Chao Luo, Visiting scientist (PhD, Atmospheric Physics, Chinese Academy of Sciences)
- Dawn Semple, PhD student (M.Phil, University of Cambridge, England)
Selected Refereed Publications>>
* denotes Gao’s students and postdocs
- Zhao*, Y, and Y. Gao, Mass size distributions of water-soluble inorganic and organic ions in size segregated aerosols over metropolitan Newark in the US East Coast, Atmospheric Environment, 10.1016/j.atmosenv.2008.01.032, 42, 4063-4078, 2008.
- Zhao*, Y, and Y. Gao, Acidic species and chloride depletion in coarse aerosol particles in the US east coast, Science of the Total Environment, doi:10.1016/j.scitotenv.2008.09.002, 407, 541-547, 2008.
- Gao, Z.Y., L.Q. Chen, and Y. Gao, Air-sea carbon fluxes and their controlling factors in the Prydz Bay in the Antarctic, Acta Oceanologica Sinica, 27 (3), 136-146, 2008.
- Xu*, N, and Y. Gao, Characterization of hematite dissolution affected by oxalate coating, kinetics and pH, Applied Geochemistry, doi:10.1016/j.apgeochem.2007.12.026, 23 (4), 783-793, 2008.
- Ayars*, J., and Y. Gao, Atmospheric nitrogen deposition to the Mullica River-Great Bay Ecosystem, Marine Environmental Research, 64, 590-600, 2007.
- Yang*, H., and Y. Gao, Air-to-sea flux of soluble iron: Is it driven more by HNO3 or SO2? - An examination in the light of dust aging, Atmospheric Chemistry and Physics Discussions, 7, 1-21, 2007.
- Gao, Y., J.R. Anderson, and X. Hua, Dust characteristics over the North Pacific observed through shipboard measurements during the ACE-Asia Experiment, Atmospheric Environment, doi:10.1016/j.atmosenv.2007.06.060, 41 (36), 7907-7922, 2007.
- Gao, Y., M. Kennish, and A.M. Flynn, Atmospheric deposition of nitrogen to New Jersey coastal waters and its implications for nutrient enrichment and biotic impacts, Journal of the Ecological Society of America, S31-S41, 2007.
- Berman-Frank, I., Y-B Chen, Y. Gao, K. Fennel, M. Follows, A. Milligan and P.G. Falkowski, Feedbacks between the nitrogen, carbon and oxygen cycles, in: Nitrogen in the Marine Environment (Editors D.J. Capone, D.A. Bronk, M.R. Mulholland and E.J. Carpenter), in press, 2006.
- Gao, Y., S-M Fan, and J. L. Sarmiento, Aeolian iron input to the ocean through precipitation scavenging: A modeling perspective and its implication for natural iron fertilization in the ocean, Journal of Geophysical Research, 108, D7, 4221, doi:10.1029/2002JD002420, 2003.
- Gao, Y., Atmospheric nitrogen deposition to Barnegat Bay, Atmospheric Environment, 36 (38), 5783-5794, 2002.
- Gao, Y., E. Nelson, M.P. Field, Q. Ding et al., Characterization of atmospheric trace elements in PM2.5 particulate matter over the New York-New Jersey harbor estuary, Atmospheric Environment, 36 (6), 1077-1086, 2002.
- Gao, Y., Y. J. Kaufman, D. Tanre, D. Kolber, and P. G. Falkowski, Seasonal distributions of aeolian iron fluxes to the global ocean, Geophysical Research Letters, 28 (1), 29-32, 2001.
- Gao, Y., and J. Anderson, Characteristics of Chinese aerosols determined by individual-particle analyses, Journal of Geophysical Research, 106, 18,037-18045, 2001.
- Gao, Y., Atmospheric chemistry and transport of Asian dust, in: The Health of the Yellow Sea (Eds. G. H. Hong, J. Zhang, and B. K. Park), 251-280, The Earth Love Publication Association, Seoul, 1998.
- Gao, Y. and R. A. Duce, The air-sea chemical exchange in coastal oceans, Advance in Earth Sciences, 6, 551-563, 1997.
- Gao, Y., R. Arimoto, R. A. Duce, M. Y. Zhou, L. Q. Chen, X. Y. Zhang, G. Y. Zhang, and Z. S. An, Temporal and spatial distribution of dust and its total deposition to the China Sea, Tellus, 49B, 172-189, 1997.
- Gao, Y, R. Arimoto, R. A. Duce, L. Q. Chen, M. Y. Zhou, and D. Y. Gu, Atmospheric non-sea-salt sulfate, nitrate, and Methanesulfonate over the China Sea, Journal of Geophysical Research, 101, 12,601-12,611, 1996.
- Gao, Y., R. Arimoto, R. A. Duce, D. S. Lee, and M. Y. Zhou, Input of atmospheric trace elements and mineral matter to the Yellow Sea during the spring of a low dust year, Journal of Geophysical Research, 97, 3767-3777, 1992.
- Gao, Y., R. Arimoto, M. T. Zhou, J. T. Merrill, and R. A. Duce, Relationships between the dust concentrations over eastern Asia and the remote North Pacific, Journal of Geophysical Research, 97, 9867-9872, 1992.